材料科学および工学ジャーナル

The role of hydrodynamic interaction in the dynamics of active dimer

Abstract

Tanwi Debnath and Pulak Kumar Ghosh

Janus particle is nano to micro meter sized entity having two distinct faces, only one of which is chemically or physically active. A class of Janus particle is called active or self-propelled Janus which can move extracting energy from environment by creating concentration or thermal gradient at the vicinity of its active surface. As active Janus particle acts as a motor for its self-propelled motion, we model an active Janus particle carrying a cargo (passive particle) to form an active dimer. To use the dimer in different purposes, such as targeted drag (cargo) delivery in medical science, the detailed knowledge about its dynamics in presence of hydrodynamic interaction is necessary. Therefore we study the 3D dynamics of the active dimer suspended in a shear flow. Using numerical simulations, we determine the diffusivity of such dimer in presence of long-range hydrodynamic interactions for different values of its self-propulsion speed and shear flow. We observe that the effect of hydrodynamic interactions is greatly enhanced under the condition that self-propulsion is strong enough to contrast the shear flow. We also numerically investigate the escape kinetics of the active dimer from a meta-stable state. Our simulation results show that the synchronization between barrier crossing events and the rotational relaxation process can enhance the escape rate to a large extent. Moreover, the hydrodynamic interaction conspicuously enhances the escape rate of the Janus-cargo dimer.